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UCoGeにおける強磁性磁気揺らぎが誘起するスピン三重項超伝導

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Title Spin-Triplet Superconductivity Induced by FerromagneticFluctuations in UCoGe( Digest_要約 )

Author(s) Hattori, Taisuke

Citation Kyoto University (京都大学)

Issue Date 2014-03-24

URL http://dx.doi.org/10.14989/doctor.k18060

Right 学位規則第9条第2項により要約公開; 許諾条件により要約は2014-12-24に公開

Type Thesis or Dissertation

Textversion none

(2)

Summary of thesis: Spin-Triplet Superconductivity

Induced by Ferromagnetic Fluctuations in UCoGe

Taisuke Hattori

Identification of pairing mechanism leading to the unconventional super-conductivity is one of the most challenging issues in condensed-matter physics. As the electron-phonon interaction in the conventional ductivity, magnetic fluctuations have been proposed to mediate supercon-ductivity, and considerable efforts have been made to unravel the relation-ship between magnetic fluctuations and superconductivity. Therefore the discovery of superconductivity in ferromagnet UGe2 under pressure in 2000

had a great impact and provided a new system where we can investigate the relationship between ferromagnetic (FM) fluctuations and superconductivity. So far, four uranium FM superconductors have been reported: UGe2, URhGe,

UIr, and UCoGe.

In these FM superconductors, UCoGe is one of the most experimentally ex-plored, because of the highest TSC ~ 0.8 K and lowest TCurie ~ 3 K at ambient

pressure1. Although the crystal structure is three dimensional, magnetic

properties possess strong Ising anisotropy with the c axis being the easy ax-is2. In addition, it is reported that the superconducting (SC) upper critical

limiting field Hc2 has also large anisotropy2,3; superconductivity survives

with the external field as large as 15 T along the a and b axes, whereas along the c axis is as small as 0.5 T. This large Hc2 along the a axis is suppressed

with a steep angle dependence when the field was tilted slightly from the a axis toward the c axis3. In addition, the superconductivity becomes robust

against the external field along the b axis when μ0H greater than 5 T is

ap-plied3. The observed characteristic Hc2 behavior is one of the mysterious

features of the superconductivity of UCoGe, and its origin would be related to the mechanism of the superconductivity. To clarify the relationship be-tween ferromagnetism and superconductivity, we have done Nuclear Quad-rupole Resonance (NQR) / Nuclear Magnetic Resonance (NMR) measure-ments on UCoGe.

The 59Co NQR signal below 1 K indicates ferromagnetism throughout the

sample volume, while the nuclear spin-lattice relaxation rate 1/T1 measured

on the FM signal decreases below TSC due to the opening of the SC gap,

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ferro-magnetism and superconductivity. Although ferromagnetism exists homo-geneously throughout the sample, the superconductivity of UCoGe would be intrinsically inhomogeneous, which might be interpreted in terms of a Self Induced Vortex state4,5.

From the angle-resolved NMR measurements we showed that longitudinal FM fluctuations along the c axis is dominant in UCoGe6. In addition, we

found that this longitudinal FM fluctuations are well tuned by the external magnetic field; The magnetic field along the c axis H||c suppresses the fluctuations drastically7, while transverse field H||b enhances the

fluctua-tions. Interestingly this tunable FM fluctuations seem to couple to the su-perconductivity strongly since the anisotropy of the FM fluctuations7 is well

scaled to that of the superconductivity3. Combined with the theoretical model

calculation, the longitudinal FM fluctuations are strongly suggested to be a SC pairing glue, concomitantly resolving the abovementioned puzzle of Hc2.

This scenario was supported by following Knight-shift measurements in the SC state. We found that 59Co Knight shift for H || a and b shows almost

constant behavior below TSC8. The observed Knight-shift results as well as

unchanged spontaneous moments in the SC state can be reasonably inter-preted with the scenario of spin-triplet superconductivity with band splitting where equal spin forms the pair with spin quantization axis parallel to the direction of spontaneous magnetization and the band splitting energy is larger than the SC gap energy.

Above experimental results strongly suggest that spin-triplet superconduc-tivity mediated by the longitudinal FM fluctuations with large band splitting is realized in UCoGe

References

[1] N. T. Huy et al., Phys. Rev. Lett. 99, 067006 (2007). [2] N. T. Huy et al., Phys. Rev. Lett. 100, 077002 (2008). [3] D. Aoki et al., J. Phys. Soc. Jpn. 78, 113709 (2009). [4] T. Ohta et al., J. Phys. Soc. Jpn. 79, 023707 (2010).

[5] T. Hattori et al., J. Phys. Soc. Jpn. Suppl. 80, SA007 (2011). [6] Y. Ihara et al., Phys. Rev. Lett. 105, 206403 (2010).

[7] T. Hattori et al., Phys. Rev. Lett. 108, 066403 (2012). [8] T. Hattori et al., Phys. Rev. B. 88, 085127 (2013).

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