第 6 章 スピン選択磁化測定
6.2 磁気コンプトンプロファイルにおける Tb の寄与と Co の寄与の分離
6.2.2 フィッティング結果
50
51
0 10 20
-500 0
500 1.2T
Pz(a.u.) Jmag(Pz)(counts)
MCP fitting Tb
Co
0 10 20
-1000 -500 0
500 0.8T
Pz(a.u.) Jmag(Pz)(counts)
MCP fitting Tb
Co
0 10 20
-1000 0
0.4T
Pz(a.u.) Jmag(Pz)(counts)
MCP fitting Tb
Co
0 10 20
-1000 -500 0
500 0.28T
Pz(a.u.) Jmag(Pz)(counts)
MCP fitting Tb
Co
0 10 20
-1000 0
0.18T
MCP fitting Tb
Co
Pz(a.u.) Jmag(Pz)(counts)
0 10 20
-1000 -500 0
500 0.8T
Pz(a.u.) Jmag(Pz)(counts)
MCP fitting Tb
Co
0 10 20
-1000 0
1.6T
Pz(a.u.) Jmag(Pz)(counts)
MCP fiting Tb
Co
0 10 20
-2000 -1000 0 1000
Pz(a.u.) Jmag(Pz)(counts)
2.5T
MCP fitting Co
Tb
#0421
52
0 10 20
-1000 0
0.06T
Jmag(Pz)(counts)
Pz(a.u.)
MCP fitting Tb
Co
0 10 20
-1000 0
-0.06T
Jmag(Pz)(counts)
Pz(a.u.)
MCP fitting Tb
Co
0 10 20
-1000 0
-0.08T
Pz(a.u.) Jmag(Pz)(counts)
MCP fitting Tb
Co
0 10 20
-1000 0
-0.18T
Jmag(Pz)(counts)
Pz(a.u.)
MCP fitting Tb
Co
0 10 20
-500 0 500
1000 -0.28T
Jmag(Pz)(counts)
Pz(a.u.)
MCP fitting Tb
Co
0 10 20
0
1000 -0.4T
Jmag(Pz)(counts)
Pz(a.u.)
MCP fitting Tb
Co
0 10 20
-500 0 500 1000
Jmag(Pz)(counts)
Pz(a.u.)
-0.8T
MCP fitting Tb
Co
0 10 20
0
1000 -1.2T
Jmag(Pz)(counts)
Pz(a.u.)
MCP fitting Tb
Co
53
0 10 20
0 500
Jmag(Pz)(counts)
Pz(a.u.)
0.3T MCP fitting Co
Tb
0 10 20
-200 0 200 400 600
Jmag(Pz)(counts)
Pz(a.u.)
0.12T MCP fitting Co
Tb
0 10 20
-200 0 200 400 600
Jmag(Pz)(counts)
Pz(a.u.)
0.6T MCP fitting Co
Tb
Fig.6.19 フィッティング結果(#0421(Tb20Co80))
0 10 20
-500 0 500
1000 -1.6T
Jmag(Pz)(counts)
Pz(a.u.)
MCP fitting Tb
Co
0 10 20
0 1000
MCP fitting Co
Tb
2.5T
Jmag(Pz)(counts)
Pz(a.u.)
#0426
0 10 20
0 500
Jmag(Pz)(counts)
Pz(a.u.)
2.0T MCP fitting Co
Tb
0 10 20
0 500
Jmag(Pz)(counts)
Pz(a.u.)
1.5T MCP fitting Co
Tb
0 10 20
0 500
Jmag(Pz)(counts)
Pz(a.u.)
1.0T MCP fitting Co
Tb
0 10 20
0 500
Pz(a.u.) Jmag(Pz)(counts)
0.02T MCP fitting Co
Tb
0 10 20
0 500
Pz(a.u.) Jmag(Pz)(counts)
0T MCP fitting Co
Tb
0 10 20
-200 0 200 400 600
Pz(a.u.) Jmag(Pz)(counts)
-0.02T MCP fitting
Co
Tb
0 10 20
-500 0
Pz(a.u.) Jmag(Pz)(counts)
-0.3T
MCP fitting Co
Tb
54
0 10 20
-300 -200 -100 0 100 200
Pz(a.u.) Jmag(Pz)(counts)
-0.12T
MCP fitting Co
Tb
55
0 10 20
-2000 -1000 0 1000
Pz(a.u.) Jmag(Pz)(counts)
2.5T
MCP fitting Co
Tb
#0917-1
0 10 20
-1000 -500 0
500 2.0T
Jmag(Pz)(counts)
Pz(a.u.)
MCP fitting Co
Tb
0 10 20
-1000 -500 0 500
Pz(a.u.) Jmag(Pz)(counts)
1.4T
MCP fitting Co
Tb
0 10 20
-500 0 500
Pz(a.u.) Jmag(Pz)(counts)
1.6T
MCP fitting Co
Tb
Fig.6.20 フィッティング結果(#0426(Tb14Co86))
0 10 20
-1000 -500 0
Pz(a.u.) Jmag(Pz)(counts)
-0.6T
MCP fitting Co
Tb
0 10 20
-1000 -500 0 500
Pz(a.u.) Jmag(Pz)(counts)
-1.0T
MCP fitting Co
Tb
0 10 20
-500 0
Pz(a.u.) Jmag(Pz)(counts)
-1.5T
MCP fitting Co
Tb
0 10 20
-1000 -500 0 500
Pz(a.u.) Jmag(Pz)(counts)
-2.0T
MCP fitting Co
Tb
56
0 10 20
-500 0 500
Pz(a.u.) Jmag(Pz)(counts)
1.2T
MCP fitting Co
Tb
0 10 20
-1000 -500 0 500
Pz(a.u.) Jmag(Pz)(counts)
1.0T
MCP fitting Co
Tb
0 10 20
-1000 -500 0 500
Pz(a.u.) Jmag(Pz)(counts)
0.75T
MCP fitting Co
Tb
0 10 20
-500 0 500
Pz(a.u.) Jmag(Pz)(counts)
0.5T
MCP fitting Co
Tb
0 10 20
-1000 0
Pz(a.u.) Jmag(Pz)(counts)
0.25T
MCP fitting Co
Tb
0 10 20
-1000 -500 0 500
Pz(a.u.)
Jmag(Pz)(counts) -0.25T
MCP fitting Co
Tb
0 10 20
-500 0 500
Pz(a.u.) Jmag(Pz)(counts)
-0.5T
MCP fitting Co
Tb
0 10 20
0 500
Pz(a.u.) Jmag(Pz)(counts)
-0.75T MCP fitting Co
Tb
57
0 10 20
0 1000
Pz(a.u.) Jmag(Pz)(counts)
-1.6T MCP fitting Co
Tb
0 10 20
-2000 -1000 0 1000
Pz(a.u.) Jmag(Pz)(counts)
2.5T
MCP fitting Co
Tb
#0917-2
0 10 20
-500 0 500
Pz(a.u.) Jmag(Pz)(counts)
2.0T
MCP fitting Co
Tb Fig.6.21 フィッティング結果(#0917-1(Tb18Co82))
0 10 20
-500 0 500
Pz(a.u.) Jmag(Pz)(counts)
-1.0T MCP fitting Co
Tb
0 10 20
-500 0 500
Pz(a.u.) Jmag(Pz)(counts)
-1.2T MCP fitting Co
Tb
0 10 20
-500 0 500 1000
Pz(a.u.) Jmag(Pz)(counts)
-1.4T MCP fitting Co
Tb
0 10 20
0 1000
Pz(a.u.) Jmag(Pz)(counts)
-1.6T MCP fitting Co
Tb
58
0 10 20
-500 0 500
Pz(a.u.)
0.05T
Jmag(Pz)(counts)
MCP fitting Co
Tb
0 10 20
-200 0 200 400
Jmag(Pz)(counts)
Pz(a.u.)
-0.05T
MCP fitting Co
Tb
0 10 20
-500 0 500
Jmag(Pz)(counts)
Pz(a.u.)
1.5T
MCP fitting Co
Tb
0 10 20
-500 0 500
Pz(a.u.) Jmag(Pz)(counts)
1.0T
MCP fitting Co
Tb
0 10 20
-500 0 500
Pz(a.u.) Jmag(Pz)(counts)
0.6T
MCP fitting Co
Tb
0 10 20
-500 0 500
Pz(a.u.) Jmag(Pz)(counts)
0.4T
MCP fitting Co
Tb
0 10 20
-500 0 500
Jmag(Pz)(counts)
Pz(a.u.)
0.25T
MCP fitting Co
Tb
0 10 20
-400 -200 0 200 400
Jmag(Pz)(counts)
Pz(a.u.)
0.15T
MCP fitting Co
Tb
59
0 10 20
-200 0 200
Pz(a.u.) Jmag(Pz)(counts)
-0.15T
MCP fitting Co
Tb
0 10 20
-500 0 500
Pz(a.u.) Jmag(Pz)(counts)
-0.4T MCP fitting Co
Tb
0 10 20
-500 0 500
Jmag(Pz)(counts)
Pz(a.u.)
-1.0T MCP fitting Co
Tb
0 10 20
-500 0 500
Jmag(Pz)(counts)
Pz(a.u.)
-2.0T MCP fitting Co
Tb
0 10 20
-400 -200 0 200
Jmag(Pz)(counts)
Pz(a.u.)
-0.25T
MCP fitting Co
Tb
0 10 20
-500 0 500
Jmag(Pz)(counts)
Pz(a.u.)
-0.6T MCP fitting Co
Tb
0 10 20
-500 0 500
Jmag(Pz)(counts)
Pz(a.u.)
-1.5T MCP fitting Co
Tb
60
0 10 20
0 1000 2000
Jmag(Pz)(counts)
Pz(a.u.)
2.5T MCP fitting Co
Tb
#0919-1
0 10 20
0 500 1000
Pz(a.u.) Jmag(Pz)(counts)
1.5T MCP fitting Co
Tb
0 10 20
0 500 1000
Pz(a.u.) Jmag(Pz)(counts)
0.6T MCP fitting
Co
Tb
0 10 20
0 500 1000
Pz(a.u.) Jmag(Pz)(counts)
0.4T MCP fitting
Co
Tb Fig.6.22 フィッティング結果(#0917-2(Tb22Co78))
0 10 20
0 500
Jmag(Pz)(counts)
Pz(a.u.)
2.0T MCP fitting Co
Tb
0 10 20
0 500
Pz(a.u.) Jmag(Pz)(counts)
1.0T MCP fitting
Co
Tb
61
0 10 20
-500 0 500 1000
Pz(a.u.) Jmag(Pz)(counts)
0.3T MCP fitting
Co
Tb
0 10 20
-500 0 500 1000
Pz(a.u.) Jmag(Pz)(counts)
0.1T MCP fitting
Co
Tb
0 10 20
-200 0 200
Jmag(Pz)(counts)
Pz(a.u.)
-0.1T MCP fitting Co
Tb
0 10 20
-400 -200 0 200
Pz(a.u.) Jmag(Pz)(counts)
-0.2T
MCP fitting Co
Tb
0 10 20
0 500
Pz(a.u.) Jmag(Pz)(counts)
0.2T MCP fitting
Co
Tb
0 10 20
-500 0
Pz(a.u.) Jmag(Pz)(counts)
-0.3T
MCP fitting Co
Tb
62
0 10 20
-1000 -500 0 500
Pz(a.u.) Jmag(Pz)(counts)
-0.4T
MCP fitting Co
Tb
0 10 20
-500 0
Pz(a.u.) Jmag(Pz)(counts)
-0.6T
MCP fitting Co
Tb
0 10 20
-1000 -500 0
Pz(a.u.) Jmag(Pz)(counts)
-1.5T
MCP fitting Co
Tb
0 10 20
-1000 -500 0
Pz(a.u.) Jmag(Pz)(counts)
-1.0T
Co Tb
MCP fitting
Fig.6.23 フィッティング結果(#0919-1(Tb13Co87))
-Jmag(Pz)(counts)
63
-2 -1 0 1 2
-2000 0 2000
Magnetic Field(T)
Magnetization(emu/cc)
#0426(Tb14Co86)
SpinTb
SpinCo
SSMH
Fig.6.24 元素別スピン選択磁化曲線(#0421) Fig.6.25元素別スピン選択磁化曲線(#0426)
Fig.6.26 元素別スピン選択磁化曲線(#0917-1) Fig.6.27元素別スピン選択磁化曲線(#0917-2)
-2 -1 0 1 2
-200 -100 0 100 200
Magnetic Field(T) Magnetization(emu/cc) #0421(Tb20Co80)
SpinTb
SpinCo
SSMH
-2 -1 0 1 2
-300 -200 -100 0 100 200 300
Magnetization(emu/cc)
Magnetic Field(T)
#0917-1(Tb18Co82)
SpinTb
SpinCo
SSMH
-2 -1 0 1 2
-400 -200 0 200 400
Magnetization(emu/cc)
Magnetic Field(T)
#0917-2(Tb22Co78)
SpinTb
SpinCo
SSMH
64 Fig.6.28 元素別スピン選択磁化曲線(#0919-1)
Fig.6.29元素別スピン選択磁化曲線(#0421) Fig.6.30元素別スピン選択磁化曲線(#0426)
Fig.6.31元素別スピン選択磁化曲線(#0917-1) Fig.6.32元素別スピン選択磁化曲線(#0917-2)
-2 -1 0 1 2
-1000 0 1000
Magnetization(emu/cc)
Magnetic Field(T)
#0919-1(Tb13Co87)
SpinTb
SpinCo
SSMH
-2 -1 0 1 2
-200 -100 0 100 200
Magnetic field(T)
Magnetization(emu/cc)
#0421(Tb20Co80) SpinTb
SpinCo
SSMH
-2 -1 0 1 2
-1000 0 1000
Magnetic field(T) Magnetization(emu/cc) #0426(Tb14Co86)
SpinTb
SpinCo
SSMH
-2 -1 0 1 2
-500 0 500
Magnetic field(T)
Magnetization(emu/cc) #0917-1(Tb18Co82)
SpinTb
SpinCo
SSMH
-2 -1 0 1 2
-400 -200 0 200 400
Magnetic field(T) Magnetization(emu/cc) #0917-2(Tb22Co78)
SpinTb
SpinCo
SSMH
65 Fig.6.33元素別スピン選択磁化曲線(#0919-1)
Fig.6.24~28、Fig.6.29~33を比較すると、①Coの軌道の磁気効果を考慮しない解析か
ら導出したスピン選択磁化曲線を分離した結果と比べ②TbCo2化合物としてのCoの軌道を 考慮する解析から導出したスピン選択磁化曲線を分離した結果は、飽和磁化が増大する試 料(#0421、#0917-1)、飽和磁化が減少する試料(#0426、#0919-1)、ほとんど変化しない試 料(#0917-2)がある。元素ごとの寄与と磁場との関連性を検討するためTbのスピン選択磁 気モーメントとCoのスピン選択磁気モーメントの比を求めたグラフをFig.6.34~38、
Fig.6.39~43に示す。Fig.6.34~38は①Coの軌道の磁気効果を考慮しない解析から導出し
たTbのスピン選択磁気モーメントとCoのスピン選択磁気モーメントの比、Fig.6.39~43 は②TbCo2化合物としてのCoの軌道を考慮する解析から導出したTbのスピン選択磁気モ ーメントとCoのスピン選択磁気モーメントの比のグラフである。
Fig.6.34 Tb,Coスピンの比(#0421) Fig.6.35 Tb,Coスピンの比(#0426)
-2 -1 0 1 2
-500 0 500
Magnetization(emu/cc)
Magnetic Field(T)
#0919-1(Tb13Co87)
SpinTb
SpinCo
SSMH
-2 -1 0 1 2
0.4 0.6 0.8 1
Magnetic field(T) Ratio,μS-Co/μS-Tb
Co3d spin/T b4f spin
#0421(Tb20Co80)
-2 -1 0 1 2
-2.5 -2 -1.5 -1
Magnetic field(T) Ratio,μS-Co/μS-Tb
#0426(Tb14Co86)
Co3d spin/T b4f spin
66
Fig.6.36 Tb,Coスピンの比(#0917-1) Fig.6.37 Tb,Coスピンの比(#0917-2)
Fig.6.38 Tb,Coスピンの比(#0919-1)
Fig.6.39 Tb,Coスピンの比(#0421) Fig.6.40 Tb,Coスピンの比(#0426)
-2 -1 0 1 2
-1.3 -1.2 -1.1 -1 -0.9
Magnetic field(T) Ratio,μS-Co/μS-Tb
#0917-1(Tb18Co82)
Co3d spin/T b4f spin
-2 -1 0 1 2
-2 -1 0
Magnetic field(T) Ratio, μS-Co/μS-Tb
#0917-2(Tb22Co78)
Co3d spin/T b4f spin
-2 -1 0 1 2
-2 -1
Magnetic Field (T) Ratio,μS-Co/μS-Tb
#0919-1(Tb13Co87)
Co3d spin/T b4f spin
-2 -1 0 1 2
-1.2 -1 -0.8
Magnetic field(T) Ratio, μS-Co/μS-Tb
#0421(Tb20Co80) Co3d spin/T b4f spin
-2 -1 0 1 2
-2.5 -2 -1.5 -1
Magnetic field(T) Ratio, μS-Co/μS-Tb
#0426(Tb14Co86)
Co3d spin/T b4f spin
67
Fig.6.41 Tb,Coスピンの比(#0917-1) Fig.6.42 Tb,Coスピンの比(#0917-2)
Fig.6.43 Tb,Coスピンの比(#0919-1)
この結果から、両解析共にTbのスピン選択磁気モーメントとCoのスピン選択磁気モー メントの比はどの磁場でもほぼ一定であることがわかる。なお、エラーバーの大きくなっ ている磁場は保磁力近傍の磁場である。また、磁化反転におけるTb、Co元素の寄与を明確 にするため、各元素の全磁化曲線を求める必要がある。